This paper is concerned with the new error analysis of a Hodge-decomposition based finite element method for the time-dependent Ginzburg-Landau equations in superconductivity. In this approach, the original equation of magnetic potential $\boldsymbol{A}$ is replaced by a new system consisting of four scalar variables. As a result, the conventional Lagrange finite element method (FEM) can be applied to problems defined on non-smooth domains. It is known that due to the low regularity of $\boldsymbol{A},$ conventional FEM, if applied to the original Ginzburg-Landau system directly, may converge to the unphysical solution. The main purpose of this paper is to establish an optimal error estimate for the order parameter in spatial direction, as previous analysis only gave a sub-optimal convergence rate analysis for all three variables due to coupling of variables. The analysis is based on a nonstandard quasi-projection for ψ and the corresponding negative-norm estimate for the classical Ritz projection. Our numerical experiments confirm the optimal convergence of $ψ_h.$